Journal of Inorganic Materials ›› 2021, Vol. 36 ›› Issue (6): 615-622.DOI: 10.15541/jim20200437
Special Issue: 【能源环境】光催化降解有机分子
• RESEARCH ARTICLE • Previous Articles Next Articles
AN Weijia1(), LI Jing1,2, WANG Shuyao1, HU Jinshan1, LIN Zaiyuan2, CUI Wenquan1(), LIU Li1, XIE Jun3, LIANG Yinghua1()
Received:
2020-08-10
Revised:
2020-11-12
Published:
2021-06-20
Online:
2020-12-10
Contact:
CUI Wenquan, professor. E-mail: wkcui@ncst.edu.cn; LIANG Yinghua, professor. E-mail: liangyh@ncst.edu.cn
About author:
AN Weijia(1989-), male, senior laboratory technician. E-mail: anweijia@ncst.edu.cn
Supported by:
CLC Number:
AN Weijia, LI Jing, WANG Shuyao, HU Jinshan, LIN Zaiyuan, CUI Wenquan, LIU Li, XIE Jun, LIANG Yinghua. Fe(III)/rGO/Bi2MoO6 Composite Photocatalyst Preparation and Phenol Degradation by Photocatalytic Fenton Synergy[J]. Journal of Inorganic Materials, 2021, 36(6): 615-622.
Fig. 3 XPS spectra of the compared composites (a) Full spectrum analysis; (b-f) XPS spectra of various element; (g) XPS spectra of valence band in Bi2MoO6
Fig. 4 (a) Phenol degradation activity by photocatalysis, Fenton, and photocatalysis-Fenton synergy, and (b) degradation rate constant over different conditions
Fig. 5 (a) Photocatalysis-Fenton synergy degradation stability test, (b) TOC removal of phenol over photocatalysis, Fenton reaction, and photocatalysis-Fenton synergy
Fig. 7 (a) Influence of degradation activity with the addition of quenchers, and (b) concentration of ?OH generated at photocatalysis, Fenton and photocatalysis-Fenton synergy
Fig. S3 Comparison of the activity of different phenol removal efficiency (a) different proportions of Fe (III) (C0 = 5 ppm); (b) Different catalyst dosages (C0 = 5 ppm, 20% Fe (III)/rGO/Bi2MoO6); (c) different amounts of hydrogen peroxide (C0 = 5 ppm, 20% Fe (III)/rGO/Bi2MoO6, catalyst concentration: 1.0 g/L); (d) different pH (C0 = 5 ppm, 20 % Fe (III)/rGO/Bi2MoO6, catalyst concentration: 1.0 g/L, H2O2 = 19.5 mmol/L) *ppm=mg/L
[1] |
ZHANG D S, CAI H, GAO K Y, et al. Preparation and visible-light photocatalytic degradation on metronidazole of Zn2SiO4-ZnO-biochar composites. Journal of Inorganic Materials, 2020,35(8):923-930.
DOI URL |
[2] |
AN W J, TIAN L Y, HU J S, et al. Efficient degradation of organic pollutants by catalytic ozonation and photocatalysis synergy system using double-functional MgO/g-C3N4 catalyst. Applied Surface Science, 2020,534:147518.
DOI URL |
[3] |
AN W J, SUN K L, HU J S, et al. The Z-scheme Ag2CO3@g-C3N4 core-shell structure for increased photoinduced charge separation and stable photocatalytic degradation. Applied Surface Science, 2020,504:144345.
DOI URL |
[4] |
HU J S, ZHANG P F, AN W J, et al. In-situ Fe-doped g-C3N4 heterogeneous catalyst via photocatalysis-Fenton reaction with enriched photocatalytic performance for removal of complex wastewater. Applied Catalysis B-Environmental, 2019,245:130-142.
DOI URL |
[5] |
DU X, ZHAO T Y, XIU Z Y, et al. Nano-zero-valent iron and MnOx selective deposition on BiVO4 decahedron superstructures for promoted spatial charge separation and exceptional catalytic activity in visible-light-driven photocatalysis-Fenton coupling system. Journal of Hazardous Materials, 2019,377:330-340.
DOI URL |
[6] |
WU Q S, YANG H P, KANG L, et al. Fe-based metal-organic frameworks as Fenton-like catalysts for highly efficient degradation of tetracycline hydrochloride over a wide pH range: acceleration of Fe(II)/Fe(III) cycle under visible light irradiation. Applied Catalysis B-Environmental, 2020,263:118282.
DOI URL |
[7] |
XU P, XU H, ZHENG D Y, et al. The efficiency and mechanism in a novel electro-Fenton process assisted by anodic photocatalysis on advanced treatment of coal gasification wastewater. Chemical Engineering Journal, 2019,361:968-974.
DOI URL |
[8] | STEFFI T, ANOOP K V, VIKAS K S, et al. Once through continuous flow removal of metronidazole by dual effect of photo- Fenton and photocatalysis in a compound parabolic concentrator at pilot plant scale. Chemical Engineering Journal, 2020,388:124184. |
[9] | XU Z M, ZHENG R, CHEN Y, et al. Ordered mesoporous Fe/TiO2 with light enhanced photo-Fenton activity. Chinese Journal of Catalysis, 2019,40:631-637. |
[10] |
HU J S, ZHANG P F, CUI J F, et al. High-efficiency removal of phenol and coking wastewater via photocatalysis-Fenton synergy over a Fe-g-C3N4 graphene hydrogel 3D structure. Journal of Industrial and Engineering Chemistry, 2020,84:305-314.
DOI URL |
[11] |
GUO L, ZHANG K L, HAN X X, et al. 2D/2D type-II Cu2ZnSnS4/Bi2WO6 heterojunctions to promote visible-light-driven photo-Fenton catalytic activity. Chinese Journal of Catalysis, 2020,41:503-513.
DOI URL |
[12] |
XING M Y, XU W J, DONG C C, et al. Metal sulfides as excellent co-catalysts for H2O2 decomposition in advanced oxidation processes. Chem, 2018,4:1359-1372.
DOI URL |
[13] |
ZHAO W H, WEI Z Q, ZHANG X D, et al. Magnetic recyclable MnFe2O4/CeO2/SnS2 ternary nano-photocatalyst for photo-Fenton degradation. Applied Catalysis A-General, 2020,593:117443.
DOI URL |
[14] |
MENG Q Q, LÜ C D, SUN J X, et al. High-efficiency Fe-Mediated Bi2MoO6 nitrogen-fixing photocatalyst: reduced surface work function and ameliorated surface reaction. Applied Catalysis B-Environmental, 2019,256:117781.
DOI URL |
[15] |
XIE Y Y, SHANG X T, LIU D, et al. Non-noble metal thickness- tunable Bi2MoO6 nanosheets for highly efficient visible-light-driven nitrobenzene reduction into aniline. Applied Catalysis B-Environmental, 2019,259:118087.
DOI URL |
[16] | WANG J L, DONG M R, ZHANG Q C, et al. Preparation of Bi2MoO6 microspheres with hollow structure and degradation performance of ofloxacin antibiotics. Chinese Journal of Inorganic Chemistry, 2020,36:827-834. |
[17] |
XIANG S W, ZHANG Z Y, WU ZHI, et al. 3D Heterostructured Ti-Based Bi2MoO6/Pd/TiO2 photocatalysts for high-efficiency solar light driven photo electrocatalytic hydrogen generation. ACS Applied Energy Materials, 2019,2:558-568.
DOI URL |
[18] | LV J L, ZHANG J F, LIU J, et al. Bi SPR-promoted Z-scheme Bi2MoO6/CdS-diethylenetriamine composite with effectively enhanced visible light photocatalytic hydrogen evolution activity and stability. ACS Sustainable Chemistry & Engineering, 2018,6:696-706. |
[19] |
XIU Z Y, CAO Y, XING Z P, et al. Wide spectral response photothermal catalysis-Fenton coupling systems with 3D hierarchical Fe3O4/Ag/Bi2MoO6 ternary hetero-superstructural magnetic microspheres for efficient high-toxic organic pollutants removal. Journal of Colloid and Interface Science, 2019,533:24-33.
DOI URL |
[20] |
JING K Q, WEN M, REN Y H, et al. Hierarchical Bi2MoO6 spheres in situ assembled by monolayer nanosheets toward photocatalytic selective oxidation of benzyl alcohol. Applied Catalysis B-Environmental, 2019,243:10-18.
DOI URL |
[21] |
WANG S Y, DING X, YANG N, et al. Insight into the effect of bromine on facet-dependent surface oxygen vacancies construction and stabilization of Bi2MoO6 for efficient photocatalytic NO removal. Applied Catalysis B-Environmental, 2020,265:118585.
DOI URL |
[22] |
HU J S, LI J, CUI J F, et al. Surface oxygen vacancies enriched FeOOH/Bi2MoO6 photocatalysis-Fenton synergy degradation of organic pollutants. Journal of Hazardous Materials, 2020,384:121399.
DOI URL |
[23] | ZHU P F, CHEN Y J, DUAN M, et al. Construction and mechanism of a highly efficient and stable Z-scheme Ag3PO4/ reduced graphene oxide/Bi2MoO6 visible-light photocatalyst. Applied Catalysis B-Environmental, 2018,8:3818-3832. |
[24] |
XUE C, LI H, AN H, et al. Cross-linked bond accelerated interfacial charge transfer in monolayer zinc indium sulfide (ZnIn2S4)/reduced graphene oxide (RGO) heterostructure for photocatalytic hydrogen production with mechanistic insight. ACS Catalysis, 2018,8:1532-1545.
DOI URL |
[25] |
LIANG Y H, WANG X, AN W J, et al. A g-C3N4@ppy-rGO 3D structure hydrogel for efficient photocatalysis. Applied Surface Science, 2019,466:666-672.
DOI URL |
[26] |
ZENG P, ZHANG Q G, PENG T Y, et al. One-pot synthesis of reduced graphene oxide-cadmium sulfide nanocomposite and its photocatalytic hydrogen production. Physical Chemistry Chemical Physics, 2011,13:21496-21502.
DOI URL |
[27] |
XU Y S, ZHANG W D. Monodispersed Ag3PO4 nanocrystals loaded on the surface of spherical Bi2MoO6 with enhanced photocatalytic performance. Dalton Transactions, 2013,42:1094-1101.
DOI URL |
[28] | YU H G, CAO G Q, CHEN FENG, et al. Enhanced photocatalytic performance of Ag3PO4 by simultaneous loading of Ag nanoparticles and Fe(III) cocatalyst. Applied Catalysis B-Environmental, 2014,160:658-665. |
[29] |
YANG L, DU C Y, TAN S Y, et al. Improved photocatalytic properties of Fe(III) ion doped Bi2MoO6 for the oxidation of organic pollutants. Ceramics International, 2021,47(4):5786-5794.
DOI URL |
[30] |
MENG X C, ZHANG Z S. Bi2MoO6 co-modified by reduced graphene oxide and palladium (PdPd2+ and Pd0) with enhanced photocatalytic decomposition of phenol. Applied Catalysis B-Environmental, 2017,209:383-393.
DOI URL |
[31] |
WANG D J, SHEN H D, GUO L, et al. Design and construction of the sandwich-like Z-scheme multicomponent CdS/Ag/Bi2MoO6 heterostructure with enhanced photocatalytic performance in RhB photodegradation. New Journal of Chemistry, 2016,40(10):8614-8624.
DOI URL |
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