Journal of Inorganic Materials ›› 2020, Vol. 35 ›› Issue (7): 735-747.DOI: 10.15541/jim20190388
Special Issue: 封面文章； 能源材料论文精选(四)：光催化与电催化(2020)； MXene材料专辑(2020~2021)； 【虚拟专辑】层状MAX，MXene及其他二维材料； 【虚拟专辑】氢能材料(2020~2021)
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LI Neng,KONG Zhouzhou,CHEN Xingzhu,YANG Yufei
Received:2019-07-25
Revised:2019-11-06
Published:2020-07-20
Online:2019-12-04
Supported by:CLC Number:
LI Neng,KONG Zhouzhou,CHEN Xingzhu,YANG Yufei. Research Progress of Novel Two-dimensional Materials in Photocatalysis and Electrocatalysis[J]. Journal of Inorganic Materials, 2020, 35(7): 735-747.
Fig. 1 Different types of two-dimensional materials[27]
Fig. 2 Structures of MAX and corresponding MXene[8]
Fig. 3 (a) ORR schematic diagram of the surface of N-doped graphene/V2C MXene composite structure[39], (b) schematic diagram of CO2RR of Mo3C2 MXene surface[41], (c) schematic diagram of N2RR of V3C2 MXene surface[42] (1 Å=0.1 nm)
Fig. 4 (a) Hydrogen adsorption free energy of V2CO2 MXene surface supported by transition metal atom[46] and (b) HER active volcano map of M3CNO2 type MXene[35]
Fig. 5 Catalytic performance modification methods of g-C3N4 (a) Different precursors and synthetic parameters affect the specific surface area and band gap of g-C3N4[6], (b) preparation of two-dimensional g-C3N4 nanosheets by nanocrystallization[60], and (c) effect of N doping on the photocatalytic hydrogen separation performance of g-C3N4[61]
Fig. 6 Side view of (a) structure of black phosphorus block to monolayer black phosphorus and its corresponding (b) band structure diagram[80]
Fig. 7 Modification of catalytic properties of two-dimensional materials (a) Boundary state regulation; (b) Functional group regulation; (c) Defect state regulation; (d) Single atomic immobilization; (e) Confinement effect; (f) Heterojunction
Fig. 8 Schematic diagram of photogenerated electron transport of (a) type I, (b) type II, (c) type III and (d) Z type heterojunction[115]
Fig. 9 Type II photocatalytic reaction mechanism of BPQD/GCN heterojunction[119]
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